Nitrogen-Doped Biomass Carbons Meet with Polyoxometalates: Synergistic Catalytic Reductant-Free Aerobic Hydroxylation of Benzene to Phenol 期刊名称： ACS Sustainable Chemistry & Engineering
二年级口算题上册作者： Long, Zhouyang,Zhang, Yadong,Chen, Guojian,Shang, Jiang,Zhou, Yu,Wang, Jun,Sun, Liming
天蓝色的彼岸读后感年份： 2019年
扔沙包教案关键词： Hydroxylation of benzene;Reductant-free;Polyoxometalate;Biomass
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carbon;Nitrogen-doped管道的故事
摘要：A nitrogen-dopedbiomass carbon catalyst SFNC(800) was preparedby carbonizing the cheap and readily available soybean flour as thestarting material at 800 °C. By combining the SFNC(800) withthe Keggin-type V-containing polyoxometalate Ch5PMoV2, a facilely recyclable catalytic system toward liquid-phareductant-free aerobic oxidation of benzene to phenol was built. Thecombined catalyst SFNC(800)-Ch5PMoV2 exhibiteda high activity with 11.2% phenol yield, 14.04 h–1 turnover frequency (TOF), and high potential for reusability underthe optimized reaction conditions. The prent
TOF value surpasdalmost all the ones of other similar previously reported reductant-freeLBTP-O2 systems and was even higher than the previous noblemetal involved system. On the basis dota船长出装
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稻田大学
